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Born in Santiago, he was the son of Manuel Barros Arana and Eugenia Borgoño Vergara. He graduated as a lawyer in 1880, held a position in the Supreme Court in 1884, was Minister of War and Navy on three occasions (1890, 1892 and 1895–96), was Minister of Foreign Affairs twice (1894 and 1918) and Finance Minister in 1901.
Barros was also an author who focused on history. He wrote several volumes including The Muzzi Mission, a Life of Admiral Patricio Lynch and Mission in the Plata, in which he defended his uncle, Diego Barros and his participation in the negotiations with Argentina over Patagonia.
