Simović played various times in Serbia's top-tier league initially with Mladost Apatin for the 2006-07 season.[2] He continued playing in the country's SuperLiga with Metalac Gornji Milanovac where he had several different stints with the club.[3][4][5] In 2012, he furthered his career in the top tier by signing with FK Radnički 1923.[6]
In the summer of 2022, he played abroad in the Canadian Soccer League with the Serbian White Eagles.[1][9] He helped the Serbs secure the regular-season title which included a playoff berth.[10] In the second round of the postseason, he played against FC Continentals where the Serbs were eliminated from the competition.[11]
Simović re-signed with the Serbs for the 2023 season where he participated in the Royal CSL Cup final where Toronto Falcons defeated the White Eagles in a penalty shootout.[12] The Serbs would finish the 2023 campaign as runners-up to Scarborough SC in the regular season.[13]
He returned for his third season and helped Serbia win the Royal CSL Cup against Scarborough.[14]
^ abVujcic, Djuradj (16 November 2022). "Re-Cap of 2022 Signings". serbianwhiteeagles.ca. Archived from the original on 4 February 2024. Retrieved 15 February 2024.