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As a young woman she witnessed the Mexican Revolution, and was present when Emiliano Zapata and his revolutionary army entered Milpa Alta in 1911. Her eyewitness account is one of the only testimonies of Emiliano Zapata speaking Nahuatl. In 1916, most of her male relatives were killed in a massacre by the Carrancistas.
In the 1930s, she served as a linguistic informant to linguists working to document the Nahuatl language. Among others she worked with Benjamin Lee Whorf who credits her in his description of Milpa Alta Nahuatl. She also worked as a model for artist Diego Rivera and her portrait can be seen in at least three of his murals, one of them the famous Tlatelolco market scene.
Charlot, John. "Jean Charlot and Luz Jiménez". English original. Published in Spanish as: Charlot, John (2007). "Jean Charlot y Luz Jiménez". Parteaguas: Revista del Instituto Cultural de Aguascalientes. 2 (8): 83–100.
Horcasitas, Fernando, ed. (1972). Life and Death in Milpa Alta: A Nahuatl chronicle of Díaz and Zapata. Narrated by Luz Jiménez. Norman: Oklahoma University Press. ISBN0-8061-1001-5.
Luz Jiménez, símbolo de un pueblo milenario, 1897–1965. México, D.F.: Consejo Nacional para la Cultura y las Artes, Inst. Nac. de Bellas Artes. 2000. ISBN970-18-3776-2. OCLC46321349.